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Zarayeneh, Neda; Kumar, Nitesh; Kalyanaraman, Ananth; Clark, Aurora E. (, Journal of Chemical Theory and Computation)
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Ding, Yu; Kumar, Nitesh; Prakash, Abhinav; Kio, Adaiyibo E.; Liu, Xin; Liu, Lei; Li, Qingchang (, Renewable Energy)null (Ed.)
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Vool, Uri; Hamo, Assaf; Varnavides, Georgios; Wang, Yaxian; Zhou, Tony X.; Kumar, Nitesh; Dovzhenko, Yuliya; Qiu, Ziwei; Garcia, Christina A.; Pierce, Andrew T.; et al (, Nature Physics)null (Ed.)
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Jaoui, Alexandre; Fauqué, Benoît; Rischau, Carl Willem; Subedi, Alaska; Fu, Chenguang; Gooth, Johannes; Kumar, Nitesh; Süß, Vicky; Maslov, Dmitrii L.; Felser, Claudia; et al (, npj Quantum Materials)Abstract The Wiedemann–Franz law establishes a link between heat and charge transport due to electrons in solids. The extent of its validity in the presence of inelastic scattering is a question raised in different contexts. Here we report on a study of the electrical, σ , and thermal, κ , conductivities in WP 2 single crystals. The Wiedemann-Franz law holds at 2 K, but a downward deviation rapidly emerges upon warming. At 13 K, there is an exceptionally large mismatch between the Lorenz number and the Sommerfeld value. We show that this is driven by a fivefold discrepancy between the T -square prefactors of electrical and thermal resistivities, both caused by electron–electron scattering. This implies the existence of abundant small-scattering-angle collisions between electrons, due to strong screening. By quantifying the relative frequency of collisions conserving momentum flux, but degrading heat flux, we identify a narrow temperature window where the hierarchy of scattering times may correspond to the hydrodynamic regime.more » « less
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